Kou Kitamura and Aoba Tsukishima are often at odds—even though their families happen to be close friends and business partners. Although the only child of a sports shop owner, Kou has never been interested in playing baseball. Despite this, he possesses an impressive batting ability honed by frequent visits to the local baseball batting center run by the Tsukushima family. On the other hand, Aoba loves to play baseball and is a star player with exceptional pitching form. However, these two seemingly complete opposites share something very important to them—Wakaba Tsukishima, Aoba's older sister and Kou's destined sweetheart. Admired by the quarrelsome duo, Wakaba often finds herself the catalyst to their never-ending rivalry. But whether or not they realize that they have more in common than either would care to admit, only time will tell. The game of baseball may just be what the pair needs to ultimately overcome their own personal struggles. [Written by MAL Rewrite]

Although already a third-year high school student, Rikka Takanashi remains a chuunibyou—a "disease" that causes people to fantasize about themselves and their surroundings. Her relationship with Yuuta Togashi has also gone unchanged for the past six months, and with entrance exams right around the corner, both of them strive to enroll at the same college. However, Tooka—Rikka's elder sister—decides to take Rikka to Italy as she has found a stable job there. This unforeseen turn of events causes a commotion between the couple as neither of them want to be separated from each other. Desperate for ideas, they seek assistance from their friends, and after a brief conversation, they come up with a plan—to elope. Chuunibyou demo Koi ga Shitai! Movie: Take On Me is a sensational drama featuring the couple—Yuuta and Rikka—as they journey across Japan. The two attempt to prevent Rikka from being taken to Italy, but will they be able to succeed in doing so?

Specials bundled with the Blu-ray/DVDs.

OVA bundled with the 14th manga volume. Story about a joint practice session between Izuku's class and Isami High students at Yuuei Academy, takes place after the field training arc in the second season.